The (original) Wicker Man - So many awesome tracks on there, especially Willows song. Great film too.
Not the whole soundtrack (can't remember any other songs of it actually!) but that song by Q Lazzerus which is playing during THAT scene in Silence of the Lambs.
Oh, Forest Gump - there are literally about 1000 classic tracks on there from the 60's and 70's! Possibly the best soundtrack ever!
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