I too was having some issues linking Entropay cards to my PayPal accounts. It was coming back saying they could not link as they could not verify address. However i found a good technique that seems to work for me.
When you add your card to PayPal, do not link it strainght away. Wait a few minutes.
The go through the profile tab and click on link my card. When it takes you to the next page wait for 1 minute before clicking on the link button. Works for me, let me know if it works for you
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